Discovery days
Contact
Prof. Dr. Matthias Wollenhaupt
Carl von Ossietzky Universität Oldenburg
Faculty V - Institute of Physics
Carl-Von-Ossietzky-Str. 9-11
D-26129 Oldenburg
Germany
Tel.: +49-441-798-3482
room: W2 1-101
matthias.wollenhaupt@uol.de
Discovery days
Ultra-fast super-continuum pulse shaping
An ultra-short laser pulse can be shaped as desired in the laboratory using spectral phase modulation. The process is based on transparent liquid crystal displays (LCD), whose individual pixels can be controlled and thus manipulated with regard to the refractive index.
In order to be able to form a laser pulse using such a display, it must first be separated into its spectral components. To do this, the laser pulse (top left in the figure, white) is directed onto a grating whose reflection angles are frequency-dependent. This results in a spatial decomposition of the laser pulse into its frequency components, or a Fourier transformation. The fanned-out beam is then collimated and directed into the so-called Fourier plane in which the above-mentioned display (black box) is located. By manipulating the refractive indices of the liquid crystal pixels (golden elements), a phase shift of the frequency components is then achieved (hence the term spectral phase shaping). The frequency components are then superimposed by a mirrored structure and a shaped pulse is created.
With a pulse shaper consisting of two liquid crystal displays whose optical axes are oriented at an angle of +-45° to the polarization of the incident laser pulse, both the spectral phase and the polarization of the laser pulse can be shaped. With the use of polarizers behind the displays, the polarization shaping can be translated into amplitude modulation. A few examples of spectral femtosecond pulse shaping are visualized below.
Pulse shaping with linear spectral phase functions
In the examples shown here, the variation of the parameter Φ of the phase function φ(ω)=Φ⋅ω is shown. The phase function is shown on the left-hand side of the monitor. There are also two polarizers behind the pulse shaper, which are used to filter out two spectral components from the overall spectrum. By varying the phase functions for the blue and red components, the two components can be delayed with respect to each other. Mathematically, this is described by the so-called group delay T(ω) (right-hand side of the monitor). The group delay is given by the derivative of the spectral phase: T(ω)=dφ(ω)/dω = Φ.
The pulse shaping with a linear phase function of the form φ(ω)= Φω is shown above. If this phase function is now shifted by the central wavelength ω0 of the laser field to be formed, i.e. the phase function φ(ω)= Φ(ω-ω0) is used, the pulse is not interferometrically shifted in time, as would be the case with arms of different lengths in an interferometer. Instead, only the so-called envelope is shifted.
Pulse shaping with quadratic spectral phase functions
In the example shown above, the variation of the parameter Φ of the phase function φ(ω)=Φ⋅ω² is visualized. Applying this phase creates a so-called chirped pulse in which the frequency components ω are linearly shifted against each other. As a result, they no longer occur simultaneously, but one after the other, whereby - depending on the sign of Φ - the chirp (chirping) can occur upwards (from low to high frequencies) or downwards (from high to low frequencies). The figure shows the progression from blue to red and thus from high to low frequencies. This is referred to as downchirp.
The linear progression of the frequency follows mathematically from the group delay T(ω). This is given by the derivative of the applied spectral phase: T(ω)=dφ(ω)/dω = Φ⋅ω. This linear shift of the frequencies is shown in the figure above directly behind the liquid crystal display by the colored blocks.
Rotation of the laser pulse with a half-wave plate
A half-wave plate is placed behind the pulse shaper. This can rotate the polarization of laser fields. The rotation of laser pulses is an essential part of photoelectroen tomography. This is described further down on this page.
Photoelectron tomography
A superachromatic half-wave plate is used to rotate the ionising polarisation-shaped laser pulse sequence. This also rotates the photoelectron wave packet. For different orientations of the electron distribution, their projection on a phosphor screen is detected and finally the 3D object is reconstructed. In the animation, actually measured projections and the tomographically reconstructed photoelectron wave packet are shown in the multiphoton ionisation of potassium atoms. If you want to understand how to design specific photoelectron wave packets with tailored light fields, have a look here: Creation of electron vortices